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Electrooxidative Amination of sp2 C–H Bonds: Coupling of Amines with Aryl Amides via Copper Catalysis
Linnaeus University, Faculty of Health and Life Sciences, Department of Chemistry and Biomedical Sciences. (Linnaeus Ctr Biomat Chem, BMC)ORCID iD: 0000-0003-0774-2528
Linnaeus University, Faculty of Health and Life Sciences, Department of Chemistry and Biomedical Sciences. (Linnaeus Ctr Biomat Chem, BMC)
Linnaeus University, Faculty of Health and Life Sciences, Department of Chemistry and Biomedical Sciences. (Linnaeus Ctr Biomat Chem, BMC)ORCID iD: 0000-0002-0407-6542
2019 (English)In: Organic Letters, ISSN 1523-7060, E-ISSN 1523-7052, Vol. 21, no 7, p. 1968-1972Article in journal (Refereed) Published
Abstract [en]

Metal-catalyzed cross-coupling reactions are among the most important transformations in organic synthesis. However, the use of C−H activation for sp2 C−N bond formation remains one of the major challenges in the field of crosscoupling chemistry. Described herein is the first example of the synergistic combination of copper catalysis and electrocatalysis for aryl C−H amination under mild reaction conditions in an atom-and step-economical manner with the liberation of H2 as the sole and benign byproduct.

Place, publisher, year, edition, pages
American Chemical Society (ACS), 2019. Vol. 21, no 7, p. 1968-1972
National Category
Organic Chemistry
Research subject
Chemistry, Organic Chemistry
Identifiers
URN: urn:nbn:se:lnu:diva-81882DOI: 10.1021/acs.orglett.9b00003ISI: 000464247500007PubMedID: 30785289Scopus ID: 2-s2.0-85062334838OAI: oai:DiVA.org:lnu-81882DiVA, id: diva2:1304332
Available from: 2019-04-12 Created: 2019-04-12 Last updated: 2019-08-29Bibliographically approved

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Kathiravan, SuppanSuriyanarayanan, SubramanianNicholls, Ian A.

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