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Harmonic transition-state theory of thermal spin transitions
University of Iceland, Iceland;St. Petersburg State University, Russia.ORCID iD: 0000-0003-3351-7172
St. Petersburg State University, Russia.
University of Iceland, Iceland.
2012 (English)In: Physical Review B. Condensed Matter and Materials Physics, ISSN 1098-0121, E-ISSN 1550-235X, Vol. 85, no 18, article id 184409Article in journal (Refereed) Published
Abstract [en]

A rate theory for thermally activated transitions in spin systems is presented. It is based on a transition-state approximation derived from Landau-Lifshitz equations of motion and quadratic expansion of the energy surface at minima and first order saddle points. While the flux out of the initial state vanishes at first order saddle points, the integrated flux over the hyperplanar transition state is nonzero and gives a rate estimate in good agreement with direct dynamical simulations of test systems over a range in damping constant. The preexponential factor obtained for transitions in model systems representing nanoclusters with 3 to 139 transition metal adatoms is on the order of 1011 to 1013s -1, similar to that of atomic rearrangements.

Place, publisher, year, edition, pages
American Physical Society, 2012. Vol. 85, no 18, article id 184409
National Category
Condensed Matter Physics
Research subject
Physics, Condensed Matter Physics
Identifiers
URN: urn:nbn:se:lnu:diva-116416DOI: 10.1103/PhysRevB.85.184409ISI: 000303794500001Scopus ID: 2-s2.0-84861125941OAI: oai:DiVA.org:lnu-116416DiVA, id: diva2:1697189
Available from: 2022-09-20 Created: 2022-09-20 Last updated: 2022-09-21Bibliographically approved

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Bessarab, Pavel F.

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