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Diyne-steered switchable regioselectivity in cobalt(ii)-catalysed C(sp(2))-H activation of amides with unsymmetrical 1,3-diynes
Linnaeus University, Faculty of Health and Life Sciences, Department of Chemistry and Biomedical Sciences. (Linnaeus Ctr Biomat Chem, BMC;BBCL)ORCID iD: 0000-0001-7683-2928
Linnaeus University, Faculty of Health and Life Sciences, Department of Chemistry and Biomedical Sciences. (Linnaeus Ctr Biomat Chem, BMC;BBCL)ORCID iD: 0000-0003-1981-4533
Linnaeus University, Faculty of Health and Life Sciences, Department of Chemistry and Biomedical Sciences. (Linnaeus Ctr Biomat Chem, BMC;BBCL)ORCID iD: 0000-0002-2042-4818
Linnaeus University, Faculty of Health and Life Sciences, Department of Chemistry and Biomedical Sciences. (Linnaeus Ctr Biomat Chem, BMC;BBCL)ORCID iD: 0000-0003-0774-2528
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2023 (English)In: Organic and biomolecular chemistry, ISSN 1477-0520, E-ISSN 1477-0539, Vol. 21, no 9, p. 1942-1951Article in journal (Refereed) Published
Abstract [en]

The regiochemical outcome of a cobalt(ii) catalysed C-H activation reaction of aminoquinoline benzamides with unsymmetrical 1,3-diynes under relatively mild reaction conditions can be steered through the choice of diyne. The choice of diyne provides access to either 3- or 4-hydroxyalkyl isoquinolinones, paving the way for the synthesis of more highly elaborate isoquinolines.

Place, publisher, year, edition, pages
Royal Society of Chemistry, 2023. Vol. 21, no 9, p. 1942-1951
National Category
Organic Chemistry
Research subject
Chemistry, Organic Chemistry
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URN: urn:nbn:se:lnu:diva-119795DOI: 10.1039/d2ob02193eISI: 000929089700001PubMedID: 36753336Scopus ID: 2-s2.0-85148443014OAI: oai:DiVA.org:lnu-119795DiVA, id: diva2:1744029
Available from: 2023-03-16 Created: 2023-03-16 Last updated: 2025-02-04Bibliographically approved

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Dhillon, PrakritiAnaspure, PrasadWiklander, Jesper G.Kathiravan, SuppanNicholls, Ian A.

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Dhillon, PrakritiAnaspure, PrasadWiklander, Jesper G.Kathiravan, SuppanNicholls, Ian A.
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Organic and biomolecular chemistry
Organic Chemistry

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