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Extreme C-13 depletion of carbonates formed during oxidation of biogenic methane in fractured granite
Linnaeus University, Faculty of Health and Life Sciences, Department of Biology and Environmental Science.ORCID iD: 0000-0001-7230-6509
Linnaeus University, Faculty of Health and Life Sciences, Department of Biology and Environmental Science.ORCID iD: 0000-0002-3585-2209
Univ Göttingen, Germany.
Stockholm University.
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2015 (English)In: Nature Communications, E-ISSN 2041-1723, Vol. 6, article id 7020Article in journal (Refereed) Published
Abstract [en]

Precipitation of exceptionally C-13-depleted authigenic carbonate is a result of, and thus a tracer for, sulphate-dependent anaerobic methane oxidation, particularly in marine sediments. Although these carbonates typically are less depleted in C-13 than in the source methane, because of incorporation of C also from other sources, they are far more depleted in C-13 (delta C-13 as light as - 69% V-PDB) than in carbonates formed where no methane is involved. Here we show that oxidation of biogenic methane in carbon-poor deep groundwater in fractured granitoid rocks has resulted in fracture-wall precipitation of the most extremely C-13-depleted carbonates ever reported, delta C-13 down to - 125% V-PDB. A microbial consortium of sulphate reducers and methane oxidizers has been involved, as revealed by biomarker signatures in the carbonates and S-isotope compositions of co-genetic sulphide. Methane formed at shallow depths has been oxidized at several hundred metres depth at the transition to a deep-seated sulphate-rich saline water. This process is so far an unrecognized terrestrial sink of methane.

Place, publisher, year, edition, pages
2015. Vol. 6, article id 7020
National Category
Microbiology
Research subject
Ecology, Microbiology
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URN: urn:nbn:se:lnu:diva-46287DOI: 10.1038/ncomms8020ISI: 000355529900003PubMedID: 25948095Scopus ID: 2-s2.0-84929180000OAI: oai:DiVA.org:lnu-46287DiVA, id: diva2:853563
Available from: 2015-09-14 Created: 2015-09-14 Last updated: 2023-03-28Bibliographically approved

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Drake, HenrikÅström, Mats E.

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