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Cooperative luminescence quenching on many-particle acceptors in disordered media
Institute of physics, Moscow.
Linnaeus University, Faculty of Science and Engineering, School of Computer Science, Physics and Mathematics. (mathematics)ORCID iD: 0000-0003-2396-6193
2012 (English)In: Physica A: Statistical Mechanics and its Applications, ISSN 0378-4371, E-ISSN 1873-2119, Vol. 391, no 12, p. 3526-3532Article in journal (Refereed) Published
Abstract [en]

Many-body cooperative energy transfer is an important process in biology, medicine, photosynthesis, rare-earth-doped laser materials, responsible for up- and down-conversion of energy, optical excitation sensitization and relaxation. We present an analytical solution for long-time asymptotic of static luminescence quenching kinetics due to cooperative energy transfer to ensembles of acceptors comprised of two-, three-, and more particles. For cooperative energy transfer and cooperative luminescence quenching to n-body acceptors we have discovered a new law of power d/(nS - (n - 1)d) time dependence (d = 1, 2, 3 is the space dimension, S = 6, 8, 10 is the multipolarty of interaction: dipole-dipole, dipole-quadrupole, or quadrupole-quadrupole). The detailed numerical simulation of cooperative quenching by Monte-Carlo method confirms the theoretical result. (C) 2012 Elsevier B.V. All rights reserved.

Place, publisher, year, edition, pages
2012. Vol. 391, no 12, p. 3526-3532
Keywords [en]
Energy transfer; Down-conversion; Rare-earth ions
National Category
Mathematics
Research subject
Natural Science, Mathematics
Identifiers
URN: urn:nbn:se:lnu:diva-19065DOI: 10.1016/j.physa.2012.02.017ISI: 000302837300018Scopus ID: 2-s2.0-84858333350OAI: oai:DiVA.org:lnu-19065DiVA, id: diva2:529328
Available from: 2012-05-30 Created: 2012-05-30 Last updated: 2018-05-16Bibliographically approved

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Basieva, Irina

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